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| 2. |
- Andersson, Klas, 1977, et al.
(författare)
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Experiments and modeling on oxy-fuel combustion chemistry during lignite-firing
- 2007
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Ingår i: The Proceedings of the 32nd International Technical Conference on Coal Utilization & Fuel Systems, Clearwater, USA, 2007.
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Konferensbidrag (övrigt vetenskapligt/konstnärligt)abstract
- This paper presents experimental and modeling work on the combustion chemistry of the oxy-fuel(O2/CO2 recycle) process with focus on the difference in NO formation between oxy-fuel and air-firedconditions. Measurements have been carried out in a 100 kW test unit, which facilitates oxy-fuelcombustion with real flue gas recycle. These measurements include in-furnace gas concentrations andtemperature profiles from lignite-fired tests. The tests comprise a reference test in air and three oxy-fuel test cases with different oxygen fractions in the recycled feed gas. Additional oxy-fuelexperiments were performed in order to study the sensitivity of the NO formation to bothstoichiometry and air ingress.The results show that for the burner settings used in this work, lignite oxy-combustion with a globaloxygen fraction of 25 vol % in the feed gas results in flame temperature levels close to those duringair-firing. Similar to previous work, it is seen that the NO emission levels in [mg/MJ] during oxy-fueloperation are reduced to less than 30 % of the emission level during air-fired conditions. The resultsfrom the modeling shows that the reduction of NO emissions during oxy-fuel combustion is caused byan increased destruction of formed and recycled NO. Further experimental tests on the OF 27condition show that an increased stoichiometric ratio (from l = 1.18 to 1.41) as well as an increasedN2 content in the feed gas (from about 1% to 15%) only has a small effect on the NO formation duringoxy-combustion.
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| 7. |
- Berntsson, Thore, 1947, et al.
(författare)
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Towards Sustainabel Oil Refinery - Pre-study for larger co-operation project
- 2008
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Rapport (övrigt vetenskapligt/konstnärligt)abstract
- In this report, the Chalmers EnergiCentrum (CEC) presents the results of a pre-study commissioned by Preem relating to the effective production of future vehicle fuels.This pre-study was made up of three studies focusing on energy streamlining, the utilisation of waste heat and carbon-dioxide separation and biorefinement relating to the gasification and hydration of vegetable oils. One of the common starting points for these studies was the current situation at the Preem refineries in Göteborg and Lysekil from where the measurement data were obtained and analysed. The report summarises the knowledge situation based on current research in the individual technical fields. The results present some interesting future opportunities for developing the sustainable production of future vehicle fuels. The sections vary, as the areas that have been examined differ and the sections have been written by different people. The reports ends with some joint conclusions and a number of questions which could be included and answered in a more extensive future main study, as part of a developed research partnership between Preem and the Chalmers University of Technology. The preliminary results of this work were analysed with the client at workshops on 1 October and 29 November 2007. The report is written in English combined with an extensive summary in Swedish including a proposal on a future main study. The study was conducted by the Chalmers EnergiCentrum (CEC), in collaboration with a number of researchers in the CEC’s network. They included Thore Berntsson, Jessica Algehed, Erik Hektor and Lennart Persson Elmeroth, all from Heat and Power Technology, Börje Gevert, Chemical and Biological Engineering, Tobias Richards, Forest Products and Chemical Engineering, Filip Johnsson and Anders Lyngfelt, Energy Technology, and Per-Åke Franck and Anders Åsblad, CIT Industriell Energianalys AB. The client, Preem, was represented by Bengt Ahlén, Sören Eriksson, Johan Jervehed, Bertil Karlsson, Gunnar Olsson, Ulf Kuylenstierna, Stefan Nyström, Martin Sjöberg and Thomas Ögren. Tobias Richards was responsible for compiling the report and Bertil Pettersson was the project manager.
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| 8. |
- Fleig, Daniel, 1980, et al.
(författare)
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Sulphur chemistry in oxy-fuel combustion
- 2009
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Ingår i: VDI-Berichte. - 0083-5560. - 9783180920566 ; 2056:24. Deutscher Flammentag, s. 289-294
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Konferensbidrag (övrigt vetenskapligt/konstnärligt)
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| 9. |
- Fleig, Daniel, 1980, et al.
(författare)
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The fate of sulphur during oxy-fuel combustion of lignite
- 2009
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Ingår i: Energy Procedia. - : Elsevier BV. - 1876-6102. ; 1:1, s. 383-390
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Konferensbidrag (övrigt vetenskapligt/konstnärligt)abstract
- This work focuses on the sulphur chemistry in oxy-fuel combustion of lignite. Comparison is made with air-fired conditions, and the main combustion products containing sulphur (ash, SO2, SO3 and H2S) are examined by modelling and experimental data. The conversion of fuel-S to SO2 is lower in oxy-fuel than in air-fuel conditions and the SO2 concentration per unit energy supplied is therefore reduced. The modelling shows that the SO3 concentration is about four times greater than the concentration in air-firing. High SO3 and H2O contents in the oxy-fuel flue gas during wet recycling increase the acid dew-point by 20 to 30 K.
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| 10. |
- Fleig, Daniel, 1980, et al.
(författare)
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The Sulphur Mass Balance in Oxy-Fuel Combustion of Lignite
- 2009
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Ingår i: 1st OXYFUEL COMBUSTION CONFERENCE: September 8-11, 2009, Cottbus, Germany.
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Konferensbidrag (övrigt vetenskapligt/konstnärligt)abstract
- This work presents an experimental study of the sulphur chemistry in oxy-fuel combustion of pulverized lignite. It has been observed that the emission of sulphur dioxide (SO2) by unit energy supplied is lower in oxy-fuel combustion than in air combustion [1-5] but the reason for this is not clear. In order to validate previous work and to clarify this difference the present work compares the amount of emitted SO2 in air and oxy-fuel combustion (wet and dry flue-gas recycle). Furthermore, the amounts of sulphur in the ash and in the water of the flue-gas condenser were determined to make a mass balance and to verify the measured amount of SO2 in the flue gas.
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